Surface fluctuations to measure the properties of complex systems in the absence of solicitation

The dynamics of thermal fluctuations of a medium reveals the properties of this medium, without the need to apply any stress. In order to exploit this principle, we have developed an optical technique for measuring spontaneous free surface height fluctuations, based on the measurement of the deflection of a laser reflected at the surface. We show that we can measure surface fluctuations of various materials, ranging from low viscosity liquids to viscoelastic solids. The viscoelastic properties of the medium probed can be determined from the experimental fluctuations spectrum. Comparing the data obtained with conventional rheometric measurements, the technique turns out to be a reliable way to characterize the rheological properties of frequencies ranging from 0.1 Hz to tens of kHz. In addition, we are interested in the influence of confinement on the surface fluctuations of a newtonian liquid. We study the effect of confinement using substrates of different types : solid plane, solid with a relief and liquid. We show that the surface fluctuations strongly depend on the substrate used. We study in particular the case where a liquid film is deposited onto a solid surface. By creating a Marangoni effect induced by a temperature gradient at the free surface of the liquid, it is possible to control the thickness of the probed film. We can therefore measure surface fluctuations of films whose thickness varies between 30 nanometers and a few micrometers. The measured spectra are sensitive to the hydrodynamic condition at the liquid-solid interface and makes it possible to estimate a possible slip length.

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Source https://theses.hal.science/tel-00936208
Author Pottier, Basile
Maintainer CCSD
Last Updated May 7, 2026, 06:29 (UTC)
Created May 7, 2026, 06:29 (UTC)
Identifier tel-00936208
Language fr
Rights https://about.hal.science/hal-authorisation-v1/
contributor Sciences et Ingénierie de la Matière Molle (SIMM) ; Université Pierre et Marie Curie - Paris 6 (UPMC)-Ecole Superieure de Physique et de Chimie Industrielles de la Ville de Paris (ESPCI Paris) ; Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-Institut de Chimie - CNRS Chimie (INC-CNRS)-Centre National de la Recherche Scientifique (CNRS)
creator Pottier, Basile
date 2013-11-26T00:00:00
harvest_object_id 360cc60c-f85f-4d6a-926c-53a48729c1c4
harvest_source_id 3374d638-d20b-4672-ba96-a23232d55657
harvest_source_title test moissonnage SELUNE
metadata_modified 2025-08-12T00:00:00
set_spec type:THESE