Among the possible solutions to build terahertz sources in the 0,2 - 2 THz range,we studied the optoelectronic way consisting in the generation of a terahertz wave by photomixingtwo laser waves at optical frequencies. The work presented in this PhD concernsthe study of dual-frequency lasers able to emit the two required waves simultaneously.We begin by developing a theoretical model describing the gain competition between thelaser modes by calculating different coupling coefficients. Experimentally, we first showthat a slight misalignment of the output mirror of the laser cavity allows to obtain a stableemission at two frequencies competing in the gain medium, which is a neodymium-dopedcrystal. Then, we focus on the pulsed regime and we show that the pulses can be synchronizedby the action of an external laser. Finally, the photomixing process has been achievedand electromagnetic waves have been generated in the radio frequencies range around 20GHz.