Study of semiconductors nanoemitters for quantum photonics: Microcavity polariton under two-photon excitation and single photon emission with colloidal nanocrystals.

My thesis focused on the study of photons and electrons con nement in several systems. First, I studied a new type of semiconductor nanocrystals to get at room temperature, an e ficient source of single photons polarized. I developed also a technique for two-photon excitation of polaritons in semiconductor microcavities. Our semiconductor nanocrystals have the particularity to have an elongated shell in cadmium sulfi de (CdS) around a spherical core of cadmium selenide (CdSe). During the last decade, semiconductor nanocrystals are known to be effi cient single photons emitters at room temperature. Their photoluminescence present two defects : Blinking, which is the phenomenon of random switching between on and o ff states, and a very low polarization issue. In this work, acting on the geometric parameters of nanocrystals (diameter of the core and length of the shell) I got strongly polarized single photon emission (linear polarization ratio greater than 80%) and showed the link between polarization and the aspect ratio of the nanocrystals. In addition, nely adjusting the thickness of the shell, I have demonstrated the possibility to reduce strongly blinking, while retaining a single photon source with high quality (g(2) < 0:2). In the second part of my thesis, I am interested in strong light-matter coupling in semiconductor microcavities and micropillars. I have developed and characterized a new type of excitation of polaritons based on two-photon absorption. In the case of micropillars where polaritons are confi ned to a 0D system, we have demonstrated photon lasing with two-photon pumping. Relaxation and interactions between polaritons are also compared under di fferent excitation.

Data and Resources

Additional Info

Field Value
Source https://theses.hal.science/tel-00818662
Author Leménager, Godefroy
Maintainer CCSD
Last Updated May 11, 2026, 07:03 (UTC)
Created May 11, 2026, 07:03 (UTC)
Identifier tel-00818662
Language fr
Rights https://about.hal.science/hal-authorisation-v1/
contributor Laboratoire Kastler Brossel (LKB (Jussieu)) ; Fédération de recherche du Département de physique de l'Ecole Normale Supérieure - ENS Paris (FRDPENS) ; École normale supérieure - Paris (ENS-PSL) ; Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-Centre National de la Recherche Scientifique (CNRS)-École normale supérieure - Paris (ENS-PSL) ; Université Paris Sciences et Lettres (PSL)-Université Paris Sciences et Lettres (PSL)-Centre National de la Recherche Scientifique (CNRS)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Centre National de la Recherche Scientifique (CNRS)
creator Leménager, Godefroy
date 2012-12-07T00:00:00
harvest_object_id d25bb99e-b63f-417d-aab8-c7fee641aec4
harvest_source_id 3374d638-d20b-4672-ba96-a23232d55657
harvest_source_title test moissonnage SELUNE
metadata_modified 2025-08-12T00:00:00
set_spec type:THESE