Influence of surface plasmons propagation on the coherence of optical systems

This experimental thesis studies effects induced by the spatial extension of surface plasmonpolaritons on the emission properties of organic and inorganic materials. First, we focused onleakage radiation microscopy images, a technic which is now widely used in a lot of differentscientific fields, as biology for exemple. We showed that the detected emission at a given point ofthe fluorescence image of an assembly of emitters mostly comes from the environment and notfrom the observed point, defining an influence circle related to the surface plasmon propagationlength. When the surface plasmon strongly interact with emitters, the strong coupling leadsto energy modifications in the system and new hybride states excitons-plasmons appear calledpolaritons. All the different localized emitters (aggregated dye chains) are not independantanymore. Diffusion measurments showed a collective effect induced by the strong-coupling.Two Young’s slits experiment added on the optical system confirm that an extended coherentstate of several micrometers is created as predicted by theory. All emitters behave as only onemacromolecule where the interaction is mediated by the surface plasmon.

Data and Resources

Additional Info

Field Value
Source https://theses.hal.science/tel-00798779
Author Aberra Guebrou, Samuel
Maintainer CCSD
Last Updated May 7, 2026, 02:01 (UTC)
Created May 7, 2026, 02:01 (UTC)
Identifier NNT: 2012LYO10217
Language fr
Rights https://about.hal.science/hal-authorisation-v1/
contributor Laboratoire de Physique de la Matière Condensée et Nanostructures (LPMCN) ; Université Claude Bernard Lyon 1 (UCBL) ; Université de Lyon-Université de Lyon-Centre National de la Recherche Scientifique (CNRS)
creator Aberra Guebrou, Samuel
date 2012-11-13T00:00:00
harvest_object_id 138dabc6-e173-482c-94d3-eff17ecdb2f9
harvest_source_id 3374d638-d20b-4672-ba96-a23232d55657
harvest_source_title test moissonnage SELUNE
metadata_modified 2026-03-31T00:00:00
set_spec type:THESE