Optical Spectroscopy of Graphite and Graphene under Megagauss Magnetic Field

Since its experimental discovery in 2004, graphene (a single layer of graphite) has attracted a lot of attention. It also leads to a renewed interest in graphite. Subsequently, both these materials have extensively been studied using different experimental techniques. In this thesis we demonstrate that transmission measurements performed in extremely high magnetic field (> 1 million times the earth's magnetic field) are a very useful tool to investigate the electronic structure of graphene and graphite. In particular, we will demonstrate that electron-hole asymmetry in graphite is caused by the often neglected free-electron kinetic energy term. This term is also present in the Hamiltonian describing electronic properties of graphene, hence it will lead to an asymmetry in graphene. Additionally, using near-infrared and visible sources from 200meV to 2eV we observe strong series of interband transitions in graphite between the four interlayer split bands (E3+, E3-, E1 and E2) up to 150 T at room temperature. The K-point electron resonances can be described well using an effective bilayer graphene model and the H-point transitions correspond to monolayer graphene. It is demonstrated that this can be reduced to a single measurement of the dispersion relation which is described by the relativistic formula where E2=m02v4 + p2v2 with v the Fermi velocity and a single particle rest energy m0v² of 385 meV for the K-point electrons and zero as expected for the H-point.

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Source https://theses.hal.science/tel-00777855
Author Solane, P. Y.
Maintainer CCSD
Last Updated May 15, 2026, 04:43 (UTC)
Created May 15, 2026, 04:43 (UTC)
Identifier tel-00777855
Language fr
Rights https://about.hal.science/hal-authorisation-v1/
contributor Laboratoire national des champs magnétiques intenses - Toulouse (LNCMI-T) ; Institut National des Sciences Appliquées - Toulouse (INSA Toulouse) ; Institut National des Sciences Appliquées (INSA)-Communauté d'universités et établissements de Toulouse (Comue de Toulouse)-Institut National des Sciences Appliquées (INSA)-Communauté d'universités et établissements de Toulouse (Comue de Toulouse)-Université Toulouse III - Paul Sabatier (UT3) ; Communauté d'universités et établissements de Toulouse (Comue de Toulouse)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])
creator Solane, P. Y.
date 2012-12-10T00:00:00
harvest_object_id e3db782b-92ff-4923-91ef-25c5e282a7dd
harvest_source_id 3374d638-d20b-4672-ba96-a23232d55657
harvest_source_title test moissonnage SELUNE
metadata_modified 2025-10-22T00:00:00
set_spec type:THESE