Optical properties of deterministic colloidal assemblies: plasmonics and dielectric confinement

Colloids - e.g. nanoparticles in solution - are objects that exhibit original optical properties. Their use as building block for fabrication of subwavelength optical components may allow novel applications in the field of integrated optics and biological detection. Anyway colloidal particles handling remains a challenge because of their small size and their random dispersion into a liquid medium. In this context, we created new colloidal optical components thanks to nanofabrication techniques based on the convective assisted capillary force assembly method. Two different kinds of structure were made and their optical behavior was studied : gold colloidal dimers and polystyrene dielectric microspheres assembled as chains or arrays. For the dimers, a fundamental study was performed on plasmonic phenomena that rule the optical properties of these objects. Next, their potential was evaluated in terms of ultrasensitive SERS sensor and also as optical nanoantenna of quantum dot emitters. For the microspheres, the propagation and scattering behaviors of whispering gallery modes that travel into the microspheres were first investigated. Their potential use as ultra- sensitive sensors was also discussed. In addition, a second study was made on the guiding properties of linear microspheres chains. In order to complete this work, one last optical component was developped in addition to the fabricated colloidal waveguides and colloidal sensors. This component is a white light microsource that was designed for applications as a versatile localized emitter for integrated optics.

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Source https://theses.hal.science/tel-00673254
Author Lecarme, Olivier
Maintainer CCSD
Last Updated May 27, 2026, 09:22 (UTC)
Created May 27, 2026, 09:22 (UTC)
Identifier tel-00673254
Language fr
Rights https://about.hal.science/hal-authorisation-v1/
contributor Laboratoire des technologies de la microélectronique (LTM) ; Université Joseph Fourier - Grenoble 1 (UJF)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Centre National de la Recherche Scientifique (CNRS)
creator Lecarme, Olivier
date 2011-12-20T00:00:00
harvest_object_id 18555812-75c9-4105-9b97-54a4790a56d2
harvest_source_id 3374d638-d20b-4672-ba96-a23232d55657
harvest_source_title test moissonnage SELUNE
metadata_modified 2025-09-27T00:00:00
set_spec type:THESE