Dynamics and Optical control of a single spin in a Quantum Dot

We have studied the dynamic properties of a single spin (Mn impurity or resident electron) in a II-VI semiconductor quantum dot. A quantum dot doped with a single Mn atom presents six lines which allow to probe optically the spin-state of the Mn atom. Pump-probe experiments at a single dot level were carried out to demonstrate that the Mn spin could be oriented in a few tens of ns, and that the spin-distribution prepared by such means was perfectly conserved over a few µs. The optical pumping of the Mn spin at zero magnetic field is controlled by a strain-induced magnetic anisotropy. Furthermore, seeking for a microscopic mechanism controlling the optical pumping of the Mn atom, we have evidenced spin relaxation channels within the exciton-Mn complex. At last, we have evidenced an optical Stark effect on any of the lines of a Mn-doped quantum dot. Concerning the dynamics of an electron in a II-VI quantum dot, we have evidenced optical pumping of the resident electron, and dynamic nuclear spin polarization.

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Source https://theses.hal.science/tel-00670963
Author Le Gall, Claire
Maintainer CCSD
Last Updated May 28, 2026, 09:24 (UTC)
Created May 28, 2026, 09:24 (UTC)
Identifier NNT: 2011GRENY057
Language fr
Rights https://about.hal.science/hal-authorisation-v1/
contributor Institut Néel (NEEL) ; Université Joseph Fourier - Grenoble 1 (UJF)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Centre National de la Recherche Scientifique (CNRS)
creator Le Gall, Claire
date 2011-11-04T00:00:00
harvest_object_id 4695704a-c043-462e-8f97-d94a9ebf96b7
harvest_source_id 3374d638-d20b-4672-ba96-a23232d55657
harvest_source_title test moissonnage SELUNE
metadata_modified 2026-03-30T00:00:00
set_spec type:THESE